Joana Vaz Pinto
Materials Science Department (DCM)
CENIMAT/I3N, Campus de Caparica Gab 1.10 (Ext 11605) (jdvp@fct.unl.pt) (email)
CENIMAT/I3N, Campus de Caparica Gab 1.10 (Ext 11605) (jdvp@fct.unl.pt) (email)
© 2017 Elsevier Ltd. Graphical abstract: The electrochemical reduction of carbon dioxide dissolved in a solution of water and ionic liquid as electrolyte, at high-pressure and near room-temperature, is reported. This work describes an electro-deposition strategy for the preparation of copper substrate cathodes, coated with bimetallic zinc-copper films, obtained from deep-eutectic solvents plating baths. The prepared bimetallic cathodes showed electrochemical activity for syngas production in 1-butyl-3-methylimidazolium triflate, with yields of 85N$μ$L (normal microliter)cm−2C−1/170N$μ$Lcm−2h−1, high selectivities, tunable H2/CO ratio and low energetic requirements.
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